Samarium(III) sulfide


Samarium sulfide is a chemical compound of the rare earth element samarium, and sulfur. In this compound samarium is in the +3 oxidation state, and sulfur is an anion in the −2 state.

Synthesis

Samarium sulfide can be produced by treating metallic samarium with sulfur:
Once prepared, samarium sulfide can be purified by chemical vapor transport using iodine.
Samarium sulfide can also be prepared by treating the sulfate with hydrogen sulfide at elevated temperatures:

Properties

The low temperature α form crystallises in the orthorhombic crystal system. The unit cell has dimensions a=7.376, b=3.9622 c=15.352 Å with volume 448.7 Å3. There are four of the formula in each unit cell. The density comes out to 5.88 kg/liter. There are two kinds of samarium coordination in the solid, one is eight coordinated with sulfur surrounding in a bicapped trigonal pyramid. The other is a sevenfold capped distorted octahedral arrangement. This structure is similar to other light rare-earth element sulfides.
Samarium sulfide is a semiconductor with a band gap of 1.7 eV. As a thin film on high area electrodes, it is under investigation as a super capacitor dielectric, with specific capacitances of up to 360 Farads per gram.

Related

Related samarium sulfides include the monosulfide SmS and the mixed valent Sm3S4 which are also semiconductors. KSm2CuS6 is a layered quaternary sulfide.